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Reactive Transport Phenomena

Analysing complex coupled thermo-hydraulical-mechanical-chemical-biological processes relevant to radionuclide release and transport in the near- and far-field of geological repositories for radioactive wastes on different scales.

The long-term evolution of the geochemical conditions in a geological repository system, the release of radionuclides from the emplaced wastes, and the radionuclide migration behaviour in the repository near- and far-field are governed by various strongly coupled thermo-hydraulical-mechanical-chemical-biological (THMCB) processes. The radionuclide transport driven either by diffusion and/or advection involves multi-phase flow phenomena under hydraulic and geochemical gradients. The transport phenomena are affected by various complex reactions including dissolution, (co)precipitation and adsorption, redox processes, and gas evolution, which are partly induced and catalysed by microbial activity.

Reactive Transport Modelling (RTM) entails the integration of hydrogeology and geo-chemistry and the prediction of chemical reactions along transport pathways in space and time. RTM has been increasingly employed in the last decades in various applications such as subsurface contaminant transport and environmental remediation, in the oil and gas industry, or in the field of radioactive waste management. However, for a rigorous comparative analyses of long-term safety aspects of geological repository systems an in-depth understanding and close to reality description of the strongly coupled THMCB processes that affect the radionuclide transport on different time and length scales is required – a so far largely unresolved scientific challenge.

Research on RTM at IEK-6 focuses on the development of complementary experimental and computational approaches to analyse and interpret the complex coupled THMC-processes relevant to radionuclide release and transport in the near- and far-field of geological repositories for radioactive wastes on different scales, employing the high performance computing (HPC) environment provided by the Jülich Supercomputing Centre (JSC) where required. This work aims at an enhanced process and system understanding across scales as well as at the reduction of uncertainties and conservatisms in performance assessments (PA), contributing thus to the scientific basis for an in-depth comparison of different repository concepts and sites as required for the German site selection procedure.

Reactive Transport ModellingConceptual hydrogeological model of a repository site (left) and simulated redox perturbation induced by the infiltration of oxygenated melt water during a glaciation event (pe after 350 years) (right).

Additional Information

Contact

Dr. Jenna Poonoosamy

Tel.: +49 2461 61-6468
Fax: +49 2461 61-2450j.poonoosamy@fz-juelich.de


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