National

AcE

Fundamental investigations of Actinide immobilization by incorporation into solid phasEs relevant for final disposal

Duration

January 2021 to December 2023

Contact

contact

Dr. Gabriel Murphy

Teamleiter für Nukleare Entsorgung Festkörperchemie

Building 05.3 / Room 337

+49 2461/61-4144

E-Mail

The AcE project aims to understand the incorporation and immobilization of actinides (An) in crystalline solid phases relevant to final disposal at the atomic level. The main objectives of the AcE project are (i) the development of synthesis strategies for An(IV)-doped solid phases, (ii) the characterization of the structural and physical properties of An-doped materials using combined atomistic and experimental approaches, and (iii) to characterize the behavior of An-doped solid phases after irradiation, e.g., long-term durability, dissolution behavior, mechanical stability, and the overall potential for An uptake in the matrix. These objectives are intended to contribute to the evaluation of innovative disposal strategies and to expand knowledge of the long-term behavior of An during disposal in deep geological repositories.

Work Package 1: Synthesis and characterization of solid phases with An(IV) and surrogates

Work Package 2: Ion irradiation and characterization of irradiated samples

Work Package 3: Understanding structure–property relationships at the atomic scale

Work Package 4: Maintenance and expansion of expertise and promotion of young researchers